Graph / DP

26 methods · 1990–2022

Graph / DP: The classical formulation: peaks become nodes in a spectrum graph whose edges are residue masses, and the peptide is the best-scoring path through it, found by dynamic programming. Nearly every classical sequencer is a version of this.

The classical formulation: peaks become nodes in a spectrum graph whose edges are residue masses, and the peptide is the best-scoring path through it, found by dynamic programming. Nearly every classical sequencer is a version of this.

The earliest of its 26 methods is Fast peptide sequencing algorithm (Bartels) (1990); 25 more have followed.

Methods 26
Papers describing them 32
Authors 130
Active 1990-06-01 to 2022-08-25
Kinds algorithm (25), adjacent
Acquisition DDA (25)

Methods (26)

Oldest first, by the paper that describes each one.

  • Fast peptide sequencing algorithm (Bartels) (1990): 1990 graph-theory algorithm that sequences polypeptides from FAB tandem mass spectra by scoring mass differences, without needing the amino acid composition, and proposes amino acid pairs or triples to bridge missing peaks. Sub-quadratic in the number of residues.
  • Sherenga (1999): Graph-theoretic de novo (foundational)
  • DP-based de novo peptide sequencing (2001): Dynamic-programming formulation over an NC-spectrum graph for de novo peptide sequencing.
  • Suboptimal de novo peptide sequencing (2003): Suboptimal-path algorithm for reporting multiple candidate de novo peptide sequences.
  • PEAKS (2003): Commercial DP-based de novo
  • DC-Novo (2004): Divide-and-conquer + spectrum simulation
  • PepNovo (2005): Probabilistic network + DP
  • AUDENS (2005): Open-source automated de novo sequencing tool with preprocessing and dynamic programming over MS/MS spectra.
  • MSNovo (2007): Mass-array dynamic programming
  • Vonode (2010): High-throughput de novo sequencing approach for high-resolution shotgun proteomics spectra.
  • pNovo (2010): First HCD-focused de novo
  • Antilope (2011): Lagrangian-relaxation formulation of de novo peptide sequencing. Frames the problem as a constrained optimization over the spectrum graph and solves it with iterative subgradient ascent.
  • PEAKS DB (2012): De-novo-assisted DB search
  • pNovo+ (2013): Complementary HCD + ETD spectra
  • UniNovo (2013): Universal de novo sequencing tool trained across fragmentation methods and instruments.
  • De novo sequencing of mixture spectra (Liu thesis) (2015): PhD work on identifying peptides from MIXTURE tandem mass spectra, where two or more peptides co-fragment: formulates the de novo problem for a mixture spectrum and solves it by dynamic programming.
  • T-Bruijn graph top-down de novo sequencing (2015): De novo sequencing from TOP-DOWN spectra, where the whole protein is fragmented rather than tryptic peptides: derives sequence tags and assembles them through a T-Bruijn graph, evaluated on carbonic anhydrase 2 and an alemtuzumab Fab.
  • UVnovo (2016): UV photodissociation de novo
  • Open-pNovo (2017): pNovo with thousands of PTMs
  • MRUniNovo (2017): Hadoop-distributed implementation of UniNovo for efficient de novo peptide sequencing.
  • Symmetric difference scoring model (2017): Scores a candidate sequence by the symmetric difference between the masses it explains and the masses actually measured, penalising an explained mass that was not observed as well as an observed mass left unexplained. Earlier scoring models only maximised the number of explained masses.
  • Retention-time-aware de novo sequencing (2018): Extends the symmetric difference scoring model with the chromatographic retention time, asking for a sequence consistent with both the fragment spectrum and the observed elution time. Develops an algorithm for each of three retention-time prediction models.
  • SWPepNovo (2019): Parallelises a PepNovo-style scoring search across the Sunway many-core architecture, using a two-level task partition and a load-balancing scheme to keep the compute elements busy. Targets the case where the spectrum dataset, not the algorithm, is the bottleneck. From the same Hunan group as MRUniNovo.
  • CycloNovo (2020): Cyclopeptide sequencing
  • MaxNovo (2021): MaxQuant spectrum-graph de novo
  • Protein Acrobat (2022): De novo peptide sequencing tool from the Cindrić group, coupling MALDI-TOF/TOF fragmentation of chemically activated peptides with de novo sequence elucidation and NCBInr alignment for organism identification (bacteria, viruses, meat-species markers).

How they score

1 of the 26 has been run on denovo_benchmarks, which ranks 17 tools over 84 datasets. The family’s best median rank is 13.

  • PEAKS: median peptide-level average precision 0.545, median rank 13 of 17

Read these next to the rest of the field, not on their own: what the numbers mean.

Papers describing them (32)

Authors (130)

Alexey Gurevich, Amanda Doherty-Kirby, Andrea Janeš, Andrew P. Horton, Andrey Prjibelski, Andrija Štajduhar, Antun Lovro Brkić, Ari Frank, Bahar Behsaz, Baozhen Shan, Bin Ma, Bing Yang, Bingwen Lu, Byung H. Park, Changjiang Xu, Chao Liu, Chengzhi Liang, Chongle Pan, Christian Bartels, Christopher Hendrie, Chuang Li, Chun-Qing Song, Debojyoti Dutta, Denis Yuen, Dustin D. Holden, Edward M. Marcotte, Ema Svetličić, Feng Lin, Fernando Vargas, Franz F. Roos, Frido Welker, George M. Church, Gilles Lajoie, Gunnar W. Klau, Haifeng Chen, Haipeng Wang, Hao Chi, Hao Yang, Hosein Mohimani, James E. Vath, Jennifer S. Brodbelt, Jianyun Liu, Jillian F. Banfield, Jing Zhang, Joe R. Cannon, John Rush, Jonas Grossmann, Joshua S. Mylne, Jürgen Cox, Kaizhong Zhang, Karl R. Clauser, Kenli Li, Keqin Li, Kira Vyatkina, Knut Reinert, Kun He, Kyowon Jeong, Larry Smarr, Le-Heng Wang, Lei Xin, Lennard J. M. Dekker, Lijuan Mo, Ljiljana Paša-Tolić, Long Wu, Lucas K. Mathis, Lucija Dončević, Ludovic Gillet, Luka Ozdanovac, Marina Čeprnja, Mario Cindrić, Mark Cieliebak, Mark Fisher, Martijn M. VanDuijn, Matthew Tepel, Matthias Müller, Meng-Qiu Dong, Michael L. Nielsen, Mikhail Dvorkin, Mikhail M. Savitski, Ming Li, Ming-Yang Kao, Mingjie Xie, Nagiza F. Samatova, Nathan C. VerBerkmoes, Nikola Tolić, Patricia A. Carey, Pavel A. Pevzner, Pelagia Kyriakidou, Peter Widmayer, Petra Gutenbrunner, Pieter C. Dorrestein, Qiang He, Robert L. Hettich, Roman A. Zubarev, Rui-Xiang Sun, Sacha Baginsky, Sandro Andreotti, Sangtae Kim, Scott A. Robotham, Si Wu, Si-Min He, Simon Rösch, Sonya Alexandrova, Tao Chen, Theo M. Luider, Theresa A. Addona, Thomas Tschager, Ting Chen, Tomas Hruz, Tomislav Tustonić, Valentin Venzin, Victoria C. Cotham, Vlado Dancík, W. Hayes McDonald, Weiming Zhang, Weiwu Chen, Wen-Feng Zeng, Wen-Jing Zhou, Wilhelm Gruissem, Xianghui Xie, Xiaowen Liu, Yan Fu, Yi Liu (Western Ontario), Yunhu Wan, Yunping Zhu, Yves Frank, Zefeng Zhang, Zhongqi Zhang, Zsuzsanna Lipták, Zuo-Fei Yuan

Seen in the charts

Back to the full map

Back to top